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Monolayer-Based Single-Photon Source in a Liquid-Helium-Free Open Cavity Featuring 65% Brightness and Quantum Coherence

  • Solid-state single-photon sources are central building blocks in quantum information processing. Atomically thin crystals have emerged as sources of nonclassical light; however, they perform below the state-of-the-art devices based on volume crystals. Here, we implement a bright single-photon source based on an atomically thin sheet of WSe2 coupled to a tunable optical cavity in a liquid-helium-free cryostat without the further need for active stabilization. Its performance is characterized by high single-photon purity (g(2)(0) = 4.7 ± 0.7%) and record-high, first-lens brightness of linearly polarized photons of 65 ± 4%, representing a decisive step toward real-world quantum applications. The high performance of our devices allows us to observe two-photon interference in a Hong–Ou–Mandel experiment with 2% visibility limited by the emitter coherence time and setup resolution. Our results thus demonstrate that the combination of the unique properties of two-dimensional materials and versatile open cavities emerges as an inspiring avenue for novel quantum optoelectronic devices.

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Metadaten
Author:Martin SiliesORCiD, Jens-Christian Drawer, Victor Nikolaevich Mitryakhin, Hangyong Shan, Sven Stephan
DOI:https://doi.org/10.1021/acs.nanolett.3c02584
ISSN:1530-6992
Parent Title (English):Nano Letters
Document Type:Article
Language:English
Year of Completion:2023
Release Date:2025/03/06
Tag:Open Microcavity; Quantum Dots; Single-Photon Source; Two-Dimensional Materials
Volume:23
Issue:18
First Page:8683
Last Page:8689
Institute:Fachbereich Technik
Research Focus Area:Nachhaltige Technologien und Prozesse