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Rabi Oscillations in Disguise: Strong Exciton-Surface Plasmon Polariton Coupling Probed by Two-Dimensional Electronic Spectroscopy

  • We explore dynamics of strong exciton-plasmon couplings using two-dimensional electronic spectra displaying pronounced Rabi oscillations of their cross-peaks. Radiative couplings govern the polariton nonlinearity and provide first access to the two-quantum-excitations of the coupled system.

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Author:Martin SiliesORCiD, Daniel Timmer, Jin-Hui Zhong, Moritz Gittinger, Thomas Quenzel
DOI:https://doi.org/10.1364/UP.2022.Th3A.5
ISBN:978-1-957171-07-4
Parent Title (English):International Conference on Ultrafast Phenomena (UP); 18.07.-22.07.2022; Montreal (Quebec Canada)
Document Type:Conference Proceeding
Language:English
Year of Completion:2022
Release Date:2025/03/06
Tag:Exciton-Surface; Oscillations; Spectroscopy
Article Number:Th3A.5
Institute:Fachbereich Technik
Research Focus Area:Nachhaltige Technologien und Prozesse